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سنتیک رهاسازی فسفر از کامپوزیت استرووایت/بیوچار تهیه شده از لجن فاضلاب خانگی | ||
تحقیقات کاربردی خاک | ||
دوره 11، شماره 2، شهریور 1402، صفحه 113-128 اصل مقاله (963.88 K) | ||
نوع مقاله: مقاله پژوهشی | ||
نویسندگان | ||
مرضیه پیری* ؛ ابراهیم سپهر | ||
دانشگاه ارومیه | ||
چکیده | ||
فاضلاب شهری به عنوان یک منبع بالقوه غنی از فسفر است. از آنجا که منابع تجدید ناپذیر سنگ فسفات در جهان محدود است لذا بازیابی فسفر از لجن فاضلاب به صورت استرووایت یا منیزیم آمونیوم فسفات (MgNH4PO4.6H2O) به عنوان کود کندرها در سراسر جهان مورد توجه قرار گرفته است. در این پژوهش رسوب فسفر از لجن فاضلاب خانگی به صورت استرووایت و کامپوزیت استرووایت/بیوچار با فرایند هضم-جذب در حضور اسید سولفوریک (2/0 نرمال) و نسبت مولی /NH4+Mg2+/PO43- 2:1:1 و pH برابر 5/8 انجام شد. بطوریکه برای تهیه استرووایت و کامپوزیت استرووایت/بیوچار از نسبتهای متفاوت بیوچار ضایعات هرس انگور به استرووایت شامل، 100:0، 75:25، 50:50 و 25:75 استفاده شد و برخی از ویژگیهای فیزیکوشیمیایی آنها مشخص گردید. سنتیک رهاسازی فسفر از نمونه ها در زمانهای 24 ساعت، 3، 5، 10، 14، 28، 42، 56 و 84 روز در آب مقطر، اسید سیتریک (20g/L ) و HCl (5/0 مولار) بررسی شد. در بررسی سنتیک نمونهها، سرعت رهاسازی عناصر فسفر، منیزیم و نیتروژن با افزایش زمان تماس نمونهها با آب، اسید سیریک و HCL افزایش یافت و داده های سنتیک در آب و اسید سیتریک برازش بهتری با معادله درجه اول (99/0-97/0=r2) و در محلول HCl برازش بهتری با معادله ایلوویچ (99/0-97/0=r2) نشان داد. نتایج آنالیز نمونهها نشان داد غلظت فلزات سنگین اندازه گیری شده در این مطالعه در حضور بیوچار افزایش یافت ولی کمتر از غلظت مجاز در کودها بود. در نتایج آنالیز XRF رسوبات بدست آمده، بیشترین ترکیب را P2O5 (28-13%) به خود اختصاص داده است. با حضور بایوچار رهاسازی فسفر، نیتروژن و منیزیم به آب، اسید سیتریک 20 گرم بر لیتر و HCl نیم مولار بیشتر شد و حداکثر حلالیت فسفر در نسبت 25:75 کامپوزیت استرووایت/بیوچار بدست آمد. بنابراین استفاده از بیوچار ضایعات هرس انگور در فرایند رسوب استرووایت موجب افزایش حلالیت و سرعت رهاسازی فسفر میگردد. | ||
کلیدواژهها | ||
بیوچار؛ لجن فاضلاب خانگی؛ فسفر؛ استروویت | ||
مراجع | ||
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